2021吉林大學化學,物理化學考研調(diào)劑信息
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學校省份：吉林
學校名稱：吉林大學
學院名稱：黃旭日、李吉來教授課題組
專業(yè)名稱：化學,物理化學
專業(yè)類型：學碩/專碩
學習方式：全日制
招收人數(shù)：1
發(fā)布渠道：網(wǎng)絡發(fā)布
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2021吉林大學化學,物理化學考研調(diào)劑信息：各位擬調(diào)劑的2021化學考生：
現(xiàn)在黃旭日、李吉來教授課題組還有1個碩士名額空缺。
請仔細閱讀一下信息，有明確意向再發(fā)郵件。
1. 只接受一志愿報考吉林大學化學學院的學生。
2. 各科都達到2021吉林大學研究生復試的初試成績基本要求
理學[07] 政治 50 外語 50 業(yè)務課一90 業(yè)務課二90
3. 跟帖無效，如有意，請發(fā)郵件 “附帶簡歷并包含考驗成績、年齡、本科院校、生源所在地、電話等信息” 至jilai--at--jlu.edu.cn
4. 謝謝，并祝各位調(diào)劑考生一切順利！good luck!
簡介如下
李吉來 博士，教授，吉林大學理論化學研究所
1977年6月生。2002年于曲阜師范大學大學獲學士學位，2007年于吉林大學大學獲博士學位。2009至2016任吉林大學副教授，2012至今任吉林大學博士生導師，2016至今任吉林大學教授。2013至今德國柏林工業(yè)大學高級訪問學者。
研究方向、主要學術成績
以國家重大需求為導向，聚焦關鍵異相催化過程相關科學問題，從分子層面理解影響復雜體系反應的關鍵因素，闡釋基元步驟反應動力學微觀本質(zhì)，并最終服務于工業(yè)催化過程的設計與優(yōu)化，實現(xiàn)能源的清潔、高效利用和無損耗轉(zhuǎn)化。通過實驗與理論的有機結合在創(chuàng)造新分子、發(fā)現(xiàn)新反應、建立新機制、提出新概念方面取得突出成果，代表性工作如下：
關聯(lián)甲烷經(jīng)典氫原子轉(zhuǎn)移中能壘與自旋密度、摻雜兩概念；首次發(fā)現(xiàn)反應誘導自旋密度定域化并激活經(jīng)典氫原子轉(zhuǎn)移；率先提出甲烷質(zhì)子耦合電子轉(zhuǎn)移機制并歸納活性位點路易斯酸堿對與能壘的內(nèi)在聯(lián)系；首次提出甲烷氫負離子轉(zhuǎn)移機理并闡明其先決條件；首次發(fā)現(xiàn)甲烷雙氫協(xié)同轉(zhuǎn)移機制，率先在離子/分子反應中率先引入外電場概念對反應機制進行本源性闡釋，提出“電誘催化”概念；探索并總結甲烷氫轉(zhuǎn)移機制的多樣性、規(guī)律性及機制間相互轉(zhuǎn)變；發(fā)現(xiàn)打破氫原子轉(zhuǎn)移機理與幾何結構關聯(lián)性的案例等。此外，在復雜體系計算方法、分子激發(fā)態(tài)、瞬時反應中間體等領域也取得標志性成果。
近五年來以第一/通訊作者發(fā)表SCI論文29篇，包括6篇J. Am. Chem. Soc.、8篇Angew. Chem. Int. Ed.和2篇Proc. Natl. Acad. Sci.。作為合作者發(fā)表其他SCI論文23篇，包括1篇J. Am. Chem. Soc.、9篇Angew. Chem. Int. Ed.和1篇 Acc. Chem. Res.。研究工作有深度、創(chuàng)新性和特色，獲得國際同行的認可，11篇論文入選雜志的封面、扉頁、VIP和熱點文章，部分原創(chuàng)性工作被國際同行譽為教科書式的發(fā)現(xiàn)。
代表作 (2015-2020)
[1] Jilai Li*, Caiyun Geng, Thomas Weiske, Mingfei Zhou*, Jun Li*, Helmut Schwarz*
Revisiting the Intriguing Electronic Features of the BeOBeC Carbyne and Some Isomers: A Quantum-Chemical Assessment
Angew. Chem. Int. Ed. 2020, 59, 17261–17265. DOI: 10.1002/anie.202007990.
[2] Jilai Li*, Caiyun Geng, Thomas Weiske, Helmut Schwarz*
On the Crucial Role of Isolated Electronic States in the Thermal Reaction of ReC+ with Dihydrogen
Angew. Chem. Int. Ed. 2020, 59, 9370-9376. DOI: 10.1002/anie.202001599
Selected as HOT Paper
[3] Jilai Li*, Caiyun Geng, Thomas Weiske, Helmut Schwarz*
Counter-intuitive Gas-phase Reactivities of [V2]+ and [V2O]+ towards CO2 Reduction: Insight from Electronic Structure Calculations
Angew. Chem. Int. Ed. 2020, 59, 12308-12314. DOI: 10.1002/anie.202001223
Highlighted as the Frontispiece article
[4] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
Complete Cleavage of the N≡N Triple Bond by Ta2N+ via Degenerate Ligand Exchange at Ambient Temperature: A Perfect Catalytic Cycle
Proc. Natl. Acad. Sci. USA 2019, 116, 21416–21420. DOI: 10.1073/pnas.1913664116
[5] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
A Reaction-Induced Localization of Spin Density Enables Thermal C–H Bond Activation of Methane by Pristine FeC4+
Chem. Eur. J. 2019, 25, 12940–12945. DOI: 10.1002/chem.201902572
Inside Cover Chem. Eur. J. 2019, 25, 12852 DOI: 10.1002/chem.201903217
[6] Caiyun Geng, Thomas Weiske, Jilai Li*, Sason Shaik*, Helmut Schwarz*
Intrinsic Reactivity of Diatomic 3d Transition-Metal Carbides in the Thermal Activation of Methane: Striking Electronic Structure Effects
J. Am. Chem. Soc. 2019, 141, 599-610. DOI: 10.1021/jacs.8b11739
[7] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
Ta2+ Mediated Ammonia Synthesis from N2 and H2 at Ambient Temperature
Proc. Natl. Acad. Sci. USA 2018, 115, 11680-11687. DOI: 10.1073/pnas.1814610115
[8] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
Thermal O–H Bond Activation of Water as Mediated by Heteronuclear [Al2Mg2O5]•+: Evidence for Oxygen-Atom Scrambling
J. Am. Chem. Soc. 2018, 140, 9275-9281. DOI: 10.1021/jacs.8b05618
[9] Helmut Schwarz*, Sason Shaik*, Jilai Li*
Electronic Effects on Room-Temperature, Gas-Phase C−H Bond Activations by Cluster Oxides and Metal Carbides: The Methane Challenge
J. Am. Chem. Soc. 2017, 139, 17201–17212. DOI: 10.1021/jacs.7b10139
[10] Lei Yue, Jilai Li*, Shaodong Zhou, Xiaoyan Sun, Maria Schlangen, Sason Shaik*, Helmut Schwarz*
Control of Product Distribution and Mechanism by Ligation and Electric Field in the Thermal Methane Activation
Angew. Chem. Int. Ed. 2017, 56, 10219–10223. DOI: 10.1002/anie.201703485
Selected as Very Important Paper & Back Cover
[11] Caiyun Geng, Jilai Li*, Thomas Weiske, Maria Schlangen, Sason Shaik*, Helmut Schwarz*
Electrostatic and Charge-Induced Methane Activation by a Concerted Double C–H Bond Insertion
J. Am. Chem. Soc. 2017, 139, 1684–1689. DOI: 10.1021/jacs.6b12514
[12] Jilai Li, Shaodong Zhou, Maria Schlangen, Thomas Weiske, Helmut Schwarz*
Hidden Hydride Transfer as a Decisive Mechanistic Step in the Reactions of the Unligated Gold Carbide [AuC]+ with Methane Under Ambient Conditions
Angew. Chem. Int. Ed. 2016, 55, 13072–13075. DOI: 10.1002/anie.201606707.
[13] Jilai Li, Shaodong Zhou, Jun Zhang, Maria Schlangen, Dandamudi Usharani, Sason Shaik, Helmut Schwarz*
Mechanistic Variants in Gas-phase Metal-oxide Mediated Activation of Methane at Ambient Conditions
J. Am. Chem. Soc. 2016, 138, 11368–11377. DOI: 10.1021/jacs.102607246
Spotlighted, DOI: 10.1021/jacs.1026b09412
[14] Jilai Li, Shaodong Zhou, Jun Zhang, Maria Schlangen, Thomas Weiske, Dandamudi Usharani, Sason Shaik*, Helmut Schwarz*
Electronic Origins of the Variable Efficiency of Room-Temperature Methane Activation by Homo- and Heteronuclear Cluster Oxide Cations [XYO2]+ (X, Y = Al, Si, Mg): Competition between Proton-Coupled Electron Transfer versus Hydrogen-Atom Transfer
J. Am. Chem. Soc. 2016, 138, 7973–7981. DOI: 10.1021/jacs.6b03798
[15] Jilai Li, Shaodong Zhou, Xiao-Nan Wu, Shiya Tang, Maria Schlangen, Helmut Schwarz*
On the Mechanisms of Hydrogen-Atom Transfer from Water to the Heteronuclear Oxide Cluster [Ga2Mg2O5]•+: Remarkable Electronic Structure Effects
Angew. Chem. Int. Ed. 2015, 54, 11861–11864. DOI: 10.1002/anie.201505336
[16] Jilai Li, Xiao-Nan Wu, Shaodong Zhou, Shiya Tang, Maria Schlangen, Helmut Schwarz*
Distinct Mechanistic Differences in the Hydrogen-Atom Transfer from Methane and Water by the Heteronuclear Oxide Cluster [Ga2MgO4]•+
Angew. Chem. Int. Ed. 2015, 54, 12298–12302. DOI: 10.1002/anie.201584261
Highlighted as frontispiece article
[17] Jilai Li, Xiao-Nan Wu, Maria Schlangen, Shaodong Zhou, Patricio González-Navarrete, Shiya Tang, Helmut Schwarz*
On the Role of the Electronic Structure of the Heteronuclear Oxide Cluster [Ga2Mg2O5]•+ in the Thermal Activation of Methane and Ethane: An Unusual Doping Effect
Angew. Chem. Int. Ed. 2015, 54, 5074-5078. DOI: 10.1002/anie.201412441
Selected as VIP
現(xiàn)在黃旭日、李吉來教授課題組還有1個碩士名額空缺。
請仔細閱讀一下信息，有明確意向再發(fā)郵件。
1. 只接受一志愿報考吉林大學化學學院的學生。
2. 各科都達到2021吉林大學研究生復試的初試成績基本要求
理學[07] 政治 50 外語 50 業(yè)務課一90 業(yè)務課二90
3. 跟帖無效，如有意，請發(fā)郵件 “附帶簡歷并包含考驗成績、年齡、本科院校、生源所在地、電話等信息” 至jilai--at--jlu.edu.cn
4. 謝謝，并祝各位調(diào)劑考生一切順利！good luck!
簡介如下
李吉來 博士，教授，吉林大學理論化學研究所
1977年6月生。2002年于曲阜師范大學大學獲學士學位，2007年于吉林大學大學獲博士學位。2009至2016任吉林大學副教授，2012至今任吉林大學博士生導師，2016至今任吉林大學教授。2013至今德國柏林工業(yè)大學高級訪問學者。
研究方向、主要學術成績
以國家重大需求為導向，聚焦關鍵異相催化過程相關科學問題，從分子層面理解影響復雜體系反應的關鍵因素，闡釋基元步驟反應動力學微觀本質(zhì)，并最終服務于工業(yè)催化過程的設計與優(yōu)化，實現(xiàn)能源的清潔、高效利用和無損耗轉(zhuǎn)化。通過實驗與理論的有機結合在創(chuàng)造新分子、發(fā)現(xiàn)新反應、建立新機制、提出新概念方面取得突出成果，代表性工作如下：
關聯(lián)甲烷經(jīng)典氫原子轉(zhuǎn)移中能壘與自旋密度、摻雜兩概念；首次發(fā)現(xiàn)反應誘導自旋密度定域化并激活經(jīng)典氫原子轉(zhuǎn)移；率先提出甲烷質(zhì)子耦合電子轉(zhuǎn)移機制并歸納活性位點路易斯酸堿對與能壘的內(nèi)在聯(lián)系；首次提出甲烷氫負離子轉(zhuǎn)移機理并闡明其先決條件；首次發(fā)現(xiàn)甲烷雙氫協(xié)同轉(zhuǎn)移機制，率先在離子/分子反應中率先引入外電場概念對反應機制進行本源性闡釋，提出“電誘催化”概念；探索并總結甲烷氫轉(zhuǎn)移機制的多樣性、規(guī)律性及機制間相互轉(zhuǎn)變；發(fā)現(xiàn)打破氫原子轉(zhuǎn)移機理與幾何結構關聯(lián)性的案例等。此外，在復雜體系計算方法、分子激發(fā)態(tài)、瞬時反應中間體等領域也取得標志性成果。
近五年來以第一/通訊作者發(fā)表SCI論文29篇，包括6篇J. Am. Chem. Soc.、8篇Angew. Chem. Int. Ed.和2篇Proc. Natl. Acad. Sci.。作為合作者發(fā)表其他SCI論文23篇，包括1篇J. Am. Chem. Soc.、9篇Angew. Chem. Int. Ed.和1篇 Acc. Chem. Res.。研究工作有深度、創(chuàng)新性和特色，獲得國際同行的認可，11篇論文入選雜志的封面、扉頁、VIP和熱點文章，部分原創(chuàng)性工作被國際同行譽為教科書式的發(fā)現(xiàn)。
代表作 (2015-2020)
[1] Jilai Li*, Caiyun Geng, Thomas Weiske, Mingfei Zhou*, Jun Li*, Helmut Schwarz*
Revisiting the Intriguing Electronic Features of the BeOBeC Carbyne and Some Isomers: A Quantum-Chemical Assessment
Angew. Chem. Int. Ed. 2020, 59, 17261–17265. DOI: 10.1002/anie.202007990.
[2] Jilai Li*, Caiyun Geng, Thomas Weiske, Helmut Schwarz*
On the Crucial Role of Isolated Electronic States in the Thermal Reaction of ReC+ with Dihydrogen
Angew. Chem. Int. Ed. 2020, 59, 9370-9376. DOI: 10.1002/anie.202001599
Selected as HOT Paper
[3] Jilai Li*, Caiyun Geng, Thomas Weiske, Helmut Schwarz*
Counter-intuitive Gas-phase Reactivities of [V2]+ and [V2O]+ towards CO2 Reduction: Insight from Electronic Structure Calculations
Angew. Chem. Int. Ed. 2020, 59, 12308-12314. DOI: 10.1002/anie.202001223
Highlighted as the Frontispiece article
[4] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
Complete Cleavage of the N≡N Triple Bond by Ta2N+ via Degenerate Ligand Exchange at Ambient Temperature: A Perfect Catalytic Cycle
Proc. Natl. Acad. Sci. USA 2019, 116, 21416–21420. DOI: 10.1073/pnas.1913664116
[5] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
A Reaction-Induced Localization of Spin Density Enables Thermal C–H Bond Activation of Methane by Pristine FeC4+
Chem. Eur. J. 2019, 25, 12940–12945. DOI: 10.1002/chem.201902572
Inside Cover Chem. Eur. J. 2019, 25, 12852 DOI: 10.1002/chem.201903217
[6] Caiyun Geng, Thomas Weiske, Jilai Li*, Sason Shaik*, Helmut Schwarz*
Intrinsic Reactivity of Diatomic 3d Transition-Metal Carbides in the Thermal Activation of Methane: Striking Electronic Structure Effects
J. Am. Chem. Soc. 2019, 141, 599-610. DOI: 10.1021/jacs.8b11739
[7] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
Ta2+ Mediated Ammonia Synthesis from N2 and H2 at Ambient Temperature
Proc. Natl. Acad. Sci. USA 2018, 115, 11680-11687. DOI: 10.1073/pnas.1814610115
[8] Caiyun Geng, Jilai Li*, Thomas Weiske, Helmut Schwarz*
Thermal O–H Bond Activation of Water as Mediated by Heteronuclear [Al2Mg2O5]•+: Evidence for Oxygen-Atom Scrambling
J. Am. Chem. Soc. 2018, 140, 9275-9281. DOI: 10.1021/jacs.8b05618
[9] Helmut Schwarz*, Sason Shaik*, Jilai Li*
Electronic Effects on Room-Temperature, Gas-Phase C−H Bond Activations by Cluster Oxides and Metal Carbides: The Methane Challenge
J. Am. Chem. Soc. 2017, 139, 17201–17212. DOI: 10.1021/jacs.7b10139
[10] Lei Yue, Jilai Li*, Shaodong Zhou, Xiaoyan Sun, Maria Schlangen, Sason Shaik*, Helmut Schwarz*
Control of Product Distribution and Mechanism by Ligation and Electric Field in the Thermal Methane Activation
Angew. Chem. Int. Ed. 2017, 56, 10219–10223. DOI: 10.1002/anie.201703485
Selected as Very Important Paper & Back Cover
[11] Caiyun Geng, Jilai Li*, Thomas Weiske, Maria Schlangen, Sason Shaik*, Helmut Schwarz*
Electrostatic and Charge-Induced Methane Activation by a Concerted Double C–H Bond Insertion
J. Am. Chem. Soc. 2017, 139, 1684–1689. DOI: 10.1021/jacs.6b12514
[12] Jilai Li, Shaodong Zhou, Maria Schlangen, Thomas Weiske, Helmut Schwarz*
Hidden Hydride Transfer as a Decisive Mechanistic Step in the Reactions of the Unligated Gold Carbide [AuC]+ with Methane Under Ambient Conditions
Angew. Chem. Int. Ed. 2016, 55, 13072–13075. DOI: 10.1002/anie.201606707.
[13] Jilai Li, Shaodong Zhou, Jun Zhang, Maria Schlangen, Dandamudi Usharani, Sason Shaik, Helmut Schwarz*
Mechanistic Variants in Gas-phase Metal-oxide Mediated Activation of Methane at Ambient Conditions
J. Am. Chem. Soc. 2016, 138, 11368–11377. DOI: 10.1021/jacs.102607246
Spotlighted, DOI: 10.1021/jacs.1026b09412
[14] Jilai Li, Shaodong Zhou, Jun Zhang, Maria Schlangen, Thomas Weiske, Dandamudi Usharani, Sason Shaik*, Helmut Schwarz*
Electronic Origins of the Variable Efficiency of Room-Temperature Methane Activation by Homo- and Heteronuclear Cluster Oxide Cations [XYO2]+ (X, Y = Al, Si, Mg): Competition between Proton-Coupled Electron Transfer versus Hydrogen-Atom Transfer
J. Am. Chem. Soc. 2016, 138, 7973–7981. DOI: 10.1021/jacs.6b03798
[15] Jilai Li, Shaodong Zhou, Xiao-Nan Wu, Shiya Tang, Maria Schlangen, Helmut Schwarz*
On the Mechanisms of Hydrogen-Atom Transfer from Water to the Heteronuclear Oxide Cluster [Ga2Mg2O5]•+: Remarkable Electronic Structure Effects
Angew. Chem. Int. Ed. 2015, 54, 11861–11864. DOI: 10.1002/anie.201505336
[16] Jilai Li, Xiao-Nan Wu, Shaodong Zhou, Shiya Tang, Maria Schlangen, Helmut Schwarz*
Distinct Mechanistic Differences in the Hydrogen-Atom Transfer from Methane and Water by the Heteronuclear Oxide Cluster [Ga2MgO4]•+
Angew. Chem. Int. Ed. 2015, 54, 12298–12302. DOI: 10.1002/anie.201584261
Highlighted as frontispiece article
[17] Jilai Li, Xiao-Nan Wu, Maria Schlangen, Shaodong Zhou, Patricio González-Navarrete, Shiya Tang, Helmut Schwarz*
On the Role of the Electronic Structure of the Heteronuclear Oxide Cluster [Ga2Mg2O5]•+ in the Thermal Activation of Methane and Ethane: An Unusual Doping Effect
Angew. Chem. Int. Ed. 2015, 54, 5074-5078. DOI: 10.1002/anie.201412441
Selected as VIP
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